高磁場下ニッケル酸化物で再入超伝導を発見 (Researchers Discover High-Field Re-entrant Superconductivity in Nickelates under High Magnetic Fields)

2026-05-11 合肥物質科学研究院(HFIPS)

香港城市大学、南方科技大学などの共同研究チームは、中国科学院の定常強磁場施設(SHMFF)を利用し、ユウロピウム(Eu)を添加した無限層ニッケル酸化物において、強磁場下で超伝導状態が再び現れる「リエントラント超伝導」を初めて観測した。通常、磁場は超伝導を破壊するが、本研究では45.22テスラの超強磁場と極低温環境下で、超伝導状態が一度消失した後、再び出現する「超伝導―常伝導―超伝導」転移を確認した。さらに、磁場方向や温度、Eu濃度によって新たな超伝導相の安定性が変化することを明らかにした。この高磁場超伝導相は、ゼロ抵抗状態と反磁性応答の双方で確認され、磁場角度0~90度でも維持される高い安定性を示した。また、従来理論のジャッカリーノ=ピーター補償機構だけでは説明できず、磁気相互作用を介した新しい電子対形成機構の可能性が示唆された。研究は、ニッケル酸化物が高温超伝導と強相関電子系研究を結び付ける重要な量子材料であることを示した。

高磁場下ニッケル酸化物で再入超伝導を発見 (Researchers Discover High-Field Re-entrant Superconductivity in Nickelates under High Magnetic Fields)
Extreme low-temperature rotational electrical transport test results under the 45 T hybrid magnet: Normalized resistance curves of highly Eu-doped SCE0.38 and SCE0.40 samples at a base temperature of 0.3 K under various magnetic field angles.(Image by MENG Wenjie)

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Euドープ無限層ニッケル酸塩における磁場再突入型超伝導 Field re-entrant superconductivity in Eu-doped infinite-layer nickelates

Mingwei Yang,Jiayin Tang,Xianfeng Wu,Heng Wang,Wenjing Xu,Haoliang Huang,Zhicheng Pei,Wenjie Meng,Guangli Kuang,Ming Yang,Jinfeng Xu,Sixia Hu,Junfeng Wang,Liang Li,Ze Wang,Chuanying Xi,Li Pi,Qingyou Lu,Ziqiang Wang,Qikun Xue,Zhuoyu Chen & Danfeng Li
Nature  Published:23 April 2026
DOI:https://doi.org/10.1038/s41586-026-10547-y  Unedited version

Abstract

Intertwined superconducting and magnetic orders may give rise to exotic quantum phases1–7, including field-induced and re-entrant superconductivity8–10. However, such magnetism-enhanced superconductivity has remained elusive in superconductors with higher transition temperatures1–3. While infinite-layer nickelates represent a new class of unconventional superconductors11–20, the impact of rare-earth magnetism on superconducting properties remains largely unexplored. Here, we show that Eu-doped infinite-layer nickelate Sm0.95−xCa0.05EuxNiO2 exhibits a magnetic-field-induced re-entrant superconducting phase in the Eu-rich over-doped regime. Zero-resistance transport and high-field diamagnetic screening confirm the superconducting nature of this phase, which emerges after the initial suppression of low-field superconductivity and remains robust across a broad range of temperatures, fields and field orientations. In the same doping range, we observe nonlinear Hall transport and hysteretic magnetoresistance, indicating the unconventional nature of the re-entrant behaviour. While partially consistent with a compensation mechanism between the Eu-derived exchange field and the applied field, our data reveal pronounced deviations from this model at the highest-doping levels. Our findings establish infinite-layer nickelates as a fertile platform for exploring magnetically driven high-field superconductivity in strongly correlated oxides.

1701物理及び化学
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