2026-04-15 東京科学大学

図1. 超格子の作製
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CsPbBr3量子ドット超格子における室温での集団点滅と光子バンチング Room temperature collective blinking and photon bunching from CsPbBr3 quantum dot superlattice
Qiwen Tan,Sudipta Seth,Boris Louis,Xiayan Wu,Nithin Pathoor,Toranosuke Takagi,Shun Omagari,Takumi Sannomiya,Johan Hofkens & Martin Vacha
Nature Communications Published:27 March 2026
DOI:https://doi.org/10.1038/s41467-026-70931-0 Unedited version
Abstract
Development of quantum systems supporting collective many-body states is crucial for advancement of quantum technologies, and perovskite quantum dots (QDs) have emerged as promising quantum light sources. However, photon bunching, a key signature of collective states, has been observed in perovskites only at cryogenic temperatures. Here, we report collective blinking and photon bunching in perovskite QD superlattices at room temperature. Sub-wavelength-sized CsPbBr3 superlattices exhibit distinct two-level blinking, and demonstrate photon bunching with a degree of up to 3.9. Time-resolved photoluminescence and super-resolution imaging reveal long lifetime components, and emission spatially confined to regions tens of nanometers in size, observations consistent with long-range exciton migration to a localized energy trap within the superlattice. Power-dependent degree of bunching and analysis of the bunching dynamics point to biexciton–exciton cascade emission as the origin of photon bunching. These findings establish perovskite QD superlattices as a promising platform for room-temperature collective optical phenomena.


