エアロゾル吸収・散乱を同時計測する統合システムを開発(Integrated System Developed for Simultaneous Measurement of Aerosol Absorption and Scattering)

2026-08-19 合肥物質科学研究院(HFIPS)

中国科学院合肥物质科学研究院の研究チームは、エアロゾルによる光の吸収と散乱を同時測定できる新たな光音響・散乱計測システムを開発した。従来は別々の試料経路や測定セルを用いるため、粒子損失や測定条件の差が生じる課題があった。新システムは単一の試料経路と共通の測定空間を採用し、積分球と音響管を組み合わせて450 nmと532 nmの2波長を同時に測定する。吸収・散乱係数に加え、Ångström指数や単一散乱アルベドも算出可能で、標準試料による校正では高い検出性能を確認した。水ミスト、燃焼エアロゾル、実大気での試験にも成功し、気候・大気質研究や長期的なエアロゾル監視への応用が期待される。

エアロゾル吸収・散乱を同時計測する統合システムを開発(Integrated System Developed for Simultaneous Measurement of Aerosol Absorption and Scattering)
Core structure of the dual-differential sphere–tube coupled photoacoustic–scattering system (Image by LI Zhengang)

<関連情報>

二重差動球管結合光音響散乱システムを用いたエアロゾル光学特性の時空間同期二波長測定 Spatiotemporally synchronized dual-wavelength measurement of aerosol optical properties using a dual-differential sphere–tube coupled photoacoustic–scattering system

Zhengang Li, Hepeng Zhang, Daming Dong, Yonghua Fang
Photoacoustics  Available online: 29 July 2026
DOI:https://doi.org/10.1016/j.pacs.2026.100864

Abstract

To reduce potential inconsistencies in particle transport, temporal response, and microenvironment in conventional split-type aerosol absorption–scattering systems, we developed a dual-wavelength spatiotemporally synchronized measurement method. Two integrating spheres serve as scattered-light collection cavities and acoustic buffers and form a low-frequency differential Helmholtz resonator, while the central tube supports a high-frequency differential second-order longitudinal mode. The 450 and 532 nm lasers were modulated at 2572 and 169 Hz and synchronously demodulated using an FPGA-based digital lock-in amplifier. Absorption channels were calibrated with NO₂, and scattering channels with N₂/CO₂ Rayleigh scattering. At 1 s integration and a 3σ criterion, the 532 nm absorption and scattering limits of detection were 1.2 and 1.32 Mm⁻¹ . Water-mist, controlled-combustion, and field tests evaluated channel isolation, relative spectral response, and ambient-operation feasibility. The system simultaneously measures dual-wavelength absorption and scattering within a common volume through a single sampling path.

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