二次元磁性体におけるトポロジカルスピン構造形成機構を解明 (Researchers Reveal How Lattice Shapes Topological Spin Structures in Two-Dimensional Magnets)

2026-05-15 合肥物質科学研究院(HFIPS)

中国科学院合肥物質科学研究院(HFIPS)の陸清友教授らの研究チームは、二次元磁性体Cr2Ge2Te6単結晶において、結晶格子がトポロジカルスピン構造の形成を直接制御することを明らかにした。研究では、定常強磁場施設を基盤に独自開発した低温・高磁場磁気力顕微鏡(MFM)を用い、三角形から八角形まで多様なスピン構造を観測した。電子スピン共鳴測定とマイクロ磁気シミュレーションの結果、これらの構造はランダムではなく、格子対称性や局所的な構造歪みに強く依存することが判明した。従来主因と考えられていたDzyaloshinskii–Moriya相互作用とは異なり、格子由来の局所エネルギー競合が安定化に重要であることを示した。また、外部磁場による構造転移や分裂・融合といった粒子的挙動も確認され、低次元磁性材料におけるトポロジカル磁性制御への新たな知見を提供した。

二次元磁性体におけるトポロジカルスピン構造形成機構を解明 (Researchers Reveal How Lattice Shapes Topological Spin Structures in Two-Dimensional Magnets)
Controllable construction and microscopic mechanism of lattice-driven topological spin structures. Selected as a cover article. (Image by FENG Qiyuan)

<関連情報>

Cr₂Ge₂Te₆単結晶における格子駆動型トポロジカルスピン構造 Lattice-Driven Topological Spin Textures in Cr2Ge2Te6 Single Crystals

Shuai Dong, Caihong Xie, Yuying Bai, Aile Wang, Zihao Li, Xuan Luo, Yuping Sun, Li Pi, Mangyuan Ma, Yongcheng Deng, Wenjie Meng, Wei Tong, Yubin Hou, Yalin Lu, Fu-Hua Sun, Qingyou Lu, Qiyuan Feng
Advanced Functional Materials  Published: 05 February 2026
DOI:https://doi.org/10.1002/adfm.74354

ABSTRACT

Owing to their unique crystal structures, van der Waals (vdW) materials provide a versatile platform for exploring emergent physical phenomena and enabling next-generation electronic and spintronic applications. However, the direct correlations between vdW crystal and intrinsic properties, such as magnetism, remain largely unexplored. Here, we demonstrate that a variety of structure-correlated topological spin textures, characterized by highly regular shapes ranging from triangles to octagons and arranged in periodic patterns, can be induced in vdW crystals. Owing to their well-resolved boundaries, the entire evolution of the quasiparticle characteristics of the topological structures, including creation, structural distortions, and collision were unambiguously revealed. More importantly, it was found that the topological annihilation occurs in an explosive manner, providing direct confirmation of the quasiparticle nature at the scale of a single magnetic unit. Simulations reveal that their formation arises from the interplay between uniaxial anisotropy and dipolar interactions, further modulated by the lattice background. These findings uncover a previously unrecognized structure-property relationship in vdW magnets and open avenues for designing and tunning of new topological spin textures.

1701物理及び化学
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