銅酸化物高温超伝導体の電子状態の全容解明と電子の分裂現象の証拠を発見

2026-02-12 上智大学

上智大学、物質・材料研究機構、京都大学、理化学研究所らの共同研究は、銅酸化物高温超伝導体Bi₂Sr₂CaCu₂O₈+δの電子状態を、角度分解光電子分光(ARPES)と走査トンネル顕微分光(QPI)データの統合解析により全エネルギー・全運動量領域で初めて解明した(Physical Review X)。単一理論模型で両実験を同時再現し、従来謎だった正のエネルギー側の運動量依存電子状態を明確化。さらに、準粒子干渉の符号構造解析から、強相関により電子が複数のフェルミ準粒子へ分裂する「電子の分数化」の実験的証拠を提示し、高温超伝導機構解明に重要な基盤を与えた。

銅酸化物高温超伝導体の電子状態の全容解明と電子の分裂現象の証拠を発見
本研究の概略。銅酸化物Bi2Sr2CaCu2O8+δについて測定された角度分解光電子分光法及び準粒子干渉効果の実験データを統合解析し、高温超伝導の鍵となる電子の分数化の実験的証拠を得た。

<関連情報>

光電子スペクトルと準粒子干渉の統合解析から得られる分数電子による銅酸化物超伝導体の統一的記述 Unified Description of Cuprate Superconductors by Fractionalized Electrons Emerging from Integrated Analyses of Photoemission Spectra and Quasiparticle Interference

Shiro Sakai, Youhei Yamaji, Fumihiro Imoto, Tsuyoshi Tamegai, Adam Kaminski, Takeshi Kondo, Yuhki Kohsaka, Tetsuo Hanaguri, and Masatoshi Imada
Physical Review X  Published: 4 February, 2026
DOI: https://doi.org/10.1103/mww7-32gn

Abstract

Electronic structure of high-temperature superconducting cuprates is studied by analyzing experimental data independently obtained from two complementary spectroscopies: one, quasiparticle interference (QPI) measured by scanning-tunneling microscopy, and the other, angle-resolved photoemission spectroscopy (ARPES). We combine these two sets of data in a unified theoretical analysis. Through explicit calculations of experimentally measurable quantities, we show that a simple two-component fermion model (TCFM) representing electron fractionalization succeeds in reproducing various detailed features of these experimental data: ARPES and QPI data are concomitantly reproduced by the TCFM in full energy and momentum spaces. The measured QPI pattern reveals a signature characteristic of the TCFM, distinct from the conventional single-component prediction, supporting the validity of the electron fractionalization in the cuprates. The integrated analysis also solves the puzzles of ARPES and QPI data that are seemingly inconsistent with each other. The overall success of the TCFM offers a comprehensive understanding of the electronic structure of the cuprates, in particular, the unoccupied side of the spectra, of which momentum-resolved structure has long been unexplored experimentally. We further predict that a characteristic QPI pattern should appear in the unoccupied high-energy part if the fractionalization is at work. We propose that integrated-spectroscopy analyses offer a promising way to explore challenging issues of strongly correlated electron systems.

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