室温下でSiC中の単一スピン情報の電気的読み出しを実現~高効率な電気的読み出しを実証し、量子デバイスの集積化に道拓く~

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2025-04-16 京都大学

京都大学化学研究所の西川哲理助教らの研究グループは、4H型炭化ケイ素(SiC)中のシリコン空孔に存在する単一電子スピンの情報を、室温下で高効率かつ電気的に読み出すことに成功した。従来困難だった単一スピンの高感度検出を、電流検出素子と光照射パターンの工夫により実現。蛍光検出(ODMR)を凌ぐ信号対雑音比を持つ光電流検出法(PDMR)の有効性も示し、量子デバイスの小型化・集積化に向けた重要な進展とされる。

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室温での炭化ケイ素中の単一スピンのコヒーレント光電気読み出し Coherent photoelectrical readout of single spins in silicon carbide at room temperature

Tetsuri Nishikawa,Naoya Morioka,Hiroshi Abe,Koichi Murata,Kazuki Okajima,Takeshi Ohshima,Hidekazu Tsuchida & Norikazu Mizuochi
Nature Communications  Published:15 April 2025
DOI:https://doi.org/10.1038/s41467-025-58629-1

室温下でSiC中の単一スピン情報の電気的読み出しを実現~高効率な電気的読み出しを実証し、量子デバイスの集積化に道拓く~

Abstract

Establishing a robust and integratable quantum system capable of sensitive qubit readout at ambient conditions is a key challenge for developing prevalent quantum technologies, including quantum networks and quantum sensing. Paramagnetic colour centres in wide bandgap semiconductors provide optical single-spin detection, yet realising efficient electrical readout technology in scalable material will unchain developing integrated ambient quantum electronics. Here, we demonstrate photoelectrical detection of single spins in silicon carbide, a material amenable to large-scale processing and electronic integration. With efficient photocarrier collection, we achieve a 1.7–2 times better signal-to-noise ratio for single spins of silicon vacancies with electrical detection than with optical detection suffering from saturating fluorescence and internal reflection. Based on our photoionisation dynamics study, further improvement would be expected with enhanced ionisation. We also observe single-defect-like features in the photocurrent image where photoluminescence is absent in the spectrum range of silicon vacancies. The efficient electrical readout in the mature material platform holds promise for developing integrated quantum devices.

1700応用理学一般
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